Activation of Mn, Li2O and LiF in the JSI TRIGA reactor to study potential tritium production monitors for fusion applications

Author:

Kodeli I.ORCID,Radulović V.,Veniger G.,Kavšek D.,Kuc T.,Ciechanowski M.,Pohorecki W.

Abstract

Abstract Two series of measurements were performed in the JSI TRIGA research reactor in 2014 and 2017 to validate the 55Mn(n,γ)56Mn cross-sections and experimentally investigate the relationship between the 55Mn(n,γ)56Mn reaction and the rate of tritium production through the 6Li(n,t)4He reaction. Indeed, previously observed similarities between the sensitivity profiles of the neutron reaction of tritium production on lithium, 6Li(n,t)4He, and those of the 55Mn(n,γ)56Mn reaction in tritium breeder modules indicated that the latter reaction could be used as an effective monitor of tritium production, at least for short-term monitoring (the half-life of 56Mn being 2.579 h). However, experimental verification, improvements and validation of the 55Mn(n,γ)56Mn cross-sections are needed in order to meet the required accuracy. Foils of certified reference material Al–1%Mn, as well as LiF thermoluminescent detectors and Li2O samples were irradiated, both bare and under cadmium, to study the potential use of the 55Mn(n,γ)56Mn reaction for monitoring tritium production in fusion devices. Additionally, Al–0.1%Au was also irradiated for comparison, the 197Au(n,γ)198Au reaction cross-section being a standard. In order to obtain complementary information for data validation purposes, the irradiations were performed in positions within the JSI TRIGA reactor with different neutron spectra, i.e. in the central channel, the pneumatic tube and the F19 position, both in the outer ‘F’ ring of the reactor core and in the IC-40 irradiation channel located in the graphite reflector surrounding the reactor core. Bare and cadmium-covered irradiations were needed to subtract the contribution of epithermal neutrons to the 55Mn(n,γ)56Mn reaction. Calculations of the reaction rates were performed using the Monte Carlo code MCNP6.1 with a detailed model of the JSI TRIGA reactor, with the samples, the irradiation capsules and covers being modelled explicitly. The uncertainties involved in the measurements and the calculations were carefully evaluated. The principal objective was to study the energy response and correlations between the 55Mn(n,γ)56Mn reaction in irradiated Al–1%Mn and the 6Li(n,t)4He reaction in irradiated LiF and Li2O. Good consistency between the measured and calculated 55Mn(n,γ)56Mn and 197Au(n,γ)198Au reaction rates, in most cases within the uncertainty bars, was observed.

Funder

Fusion for Energy

Publisher

IOP Publishing

Subject

Condensed Matter Physics,Nuclear and High Energy Physics

Reference20 articles.

1. Sensitivity and uncertainty analysis of the HCLL breeder blanket experiment in the frame of the EU fusion technology programme;Kodeli;Nucl. Eng. Des.,2011

2. TRIGA irradiations of Mn foils and TLD as potential tritium production monitors for fusion applications;Kodeli,2014

3. Neutronics experiments for uncertainty assessment of tritium breeding in HCPB and HCLL blanket mock-ups irradiated with 14 MeV neutrons;Batistoni;Nucl. Fusion,2012

4. Validation of IRDFF-v1.04 (&v1.05) dosimetry library using SINBAD shielding benchmark experiments;Kodeli,2015

5. Transport, sensitivity and uncertainty analysis of FNG 14 MeV neutron bulk shield experiment;Kodeli;J. Nucl. Sci. Technol. Suppl.,2000

Cited by 2 articles. 订阅此论文施引文献 订阅此论文施引文献,注册后可以免费订阅5篇论文的施引文献,订阅后可以查看论文全部施引文献

同舟云学术

1.学者识别学者识别

2.学术分析学术分析

3.人才评估人才评估

"同舟云学术"是以全球学者为主线,采集、加工和组织学术论文而形成的新型学术文献查询和分析系统,可以对全球学者进行文献检索和人才价值评估。用户可以通过关注某些学科领域的顶尖人物而持续追踪该领域的学科进展和研究前沿。经过近期的数据扩容,当前同舟云学术共收录了国内外主流学术期刊6万余种,收集的期刊论文及会议论文总量共计约1.5亿篇,并以每天添加12000余篇中外论文的速度递增。我们也可以为用户提供个性化、定制化的学者数据。欢迎来电咨询!咨询电话:010-8811{复制后删除}0370

www.globalauthorid.com

TOP

Copyright © 2019-2024 北京同舟云网络信息技术有限公司
京公网安备11010802033243号  京ICP备18003416号-3