Dependence of the nonlinear optical response of CdSe nanoscrolls on coating with oleic or acetic acid

Abstract

Abstract The photoluminescence and nonlinear transmission of atomically thin population of colloidal CdSe rolled-up nanosheets were investigated at the one-photon stationary excitations of excitons by the third harmonic of Nd3+:YAP laser pulses. It was revealed that the nonlinear optical response of the nanoscrolls is strongly influenced by multiwalled rolled-up structure. The broadening of exciton band and the red shift of the photoluminescence were observed and explained by coupling effect within the folded scroll-layers.