The catalytic efficiency of Ru/Mn/Ce-Al2O3 in the reduction of HCN in dry methane reforming with CO2 assisted by non-thermal plasma

Author:

Kok David Hong Kian,Ibrahim Raja Kamarulzaman Raja,Toemen Susilawati,Bakar Mohd Bakri

Abstract

Abstract This study investigates the catalytic activity of Ru/Mn/Ce-Al2O3 in eliminating HCN via dry reforming CH4 with CO2 in the packed-bed dielectric barrier discharge non-thermal plasma (DBD NTP). A packed bed DBD configuration method was carried out in the non-thermal plasma with Ru/Mn/Ce-Al2O3 catalyst, whereby BaTiO3 beads was the dielectric medium. The carrier gas for dry methane reforming was N2, the peak-to-peak voltage was 24 kV and the total flow rate was 100 sccm with a ratio of 5:5:90 (CH4:CO2:N2), respectively. Gaseous products and by-products were analysed by Fourier transform infra-red (FTIR) spectroscopy. Experimental results revealed that Ru/Mn/Ce-Al2O3 catalyst could eliminate HCN at approximately 82% and had a low selectivity in decomposing NH3. Besides, the conversion of CH4 achieved was approximately 68%.

Publisher

IOP Publishing

Subject

Computer Science Applications,History,Education

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