New evidence for CH4 enhancement in the upper troposphere associated with the Asian summer monsoon

Abstract

Abstract The Asian summer monsoon (ASM) region is a key region transporting air to the upper troposphere (UT), significantly influencing the distribution and concentration of trace gases, including methane (CH4), an important greenhouse gas. We investigate the seasonal enhancement of CH4 in the UT over the ASM region, utilizing retrievals from the Atmospheric Infrared Sounder (AIRS), model simulations and in-situ measurements. Both the AIRS data and model simulation reveal a substantial enhancement in CH4 concentrations within the active monsoon region of up to 3%, referring to the zonal means, and of up to 6% relative to the pre-monsoon season. Notably, the spatial distribution of the CH4 plume demonstrates a southwestward shift in the AIRS retrievals, in contrast to the model simulations, which predict a broader enhancement, including a significant increase to the east. A cross-comparison with in-situ measurements, including AirCore measurements over the Tibetan Plateau and airline sampling across the ASM anticyclone (ASMA), favors the enhancement represented by model simulation. Remarkable CH4 enhancement over the west Pacific is also evidenced by in-situ data and simulation as a dynamical extension of the ASMA. Our findings underscore the necessity for cautious interpretation of satellite-derived CH4 distributions, and highlight the critical role of in-situ data in anchoring the assimilation of CH4.