2022 roadmap on low temperature electrochemical CO2 reduction

Author:

Stephens Ifan E LORCID,Chan KarenORCID,Bagger AlexanderORCID,Boettcher Shannon WORCID,Bonin JulienORCID,Boutin EtienneORCID,Buckley Aya K,Buonsanti RaffaellaORCID,Cave Etosha R,Chang XiaoxiaORCID,Chee See WeeORCID,da Silva Alisson H MORCID,de Luna PhilORCID,Einsle OliverORCID,Endrődi BalázsORCID,Escudero-Escribano MariaORCID,Ferreira de Araujo Jorge VORCID,Figueiredo Marta CORCID,Hahn ChristopherORCID,Hansen Kentaro U,Haussener SophiaORCID,Hunegnaw SaraORCID,Huo Ziyang,Hwang Yun JeongORCID,Janáky CsabaORCID,Jayathilake Buddhinie SORCID,Jiao FengORCID,Jovanov Zarko P,Karimi Parisa,Koper Marc T M,Kuhl Kendra PORCID,Lee Woong HeeORCID,Liang Zhiqin,Liu Xuan,Ma SichaoORCID,Ma MingORCID,Oh Hyung-SukORCID,Robert MarcORCID,Cuenya Beatriz RoldanORCID,Rossmeisl JanORCID,Roy Claudie,Ryan Mary PORCID,Sargent Edward H,Sebastián-Pascual PaulaORCID,Seger BrianORCID,Steier LudmillaORCID,Strasser Peter,Varela Ana SofiaORCID,Vos Rafaël E,Wang XueORCID,Xu BingjunORCID,Yadegari HosseinORCID,Zhou YuxiangORCID

Abstract

Abstract Electrochemical CO2 reduction (CO2R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO2R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle.

Funder

Ministry of Economic Affairs

PPP

BV and the Dutch Research Council

Research Program of the Materials

DFF-Research Project

Villum Foundation

Institut Universitaire de France

French National Agency

CONACyT

GRANT

National Research Council Canada

European Union

SCOUTS

Laboratory Directed Research and Development

Lawrence Livermore National Laboratory

U.S. Department of Energy

Challenge Program

European Community

Korea government

NRF

National Research Foundation of Korea

Beijing National Laboratory for Molecular Sciences

DFG, German Research Foundation

Liquid Sunlight Alliance

Fuel Cell Technologies Office

Office of Energy Efficiency and Renewable Energy

Xi’an Jiaotong University

Swiss National Science Foundation

National Centre of Competence

European Research Council

Deutsche Forschungsgemeinschaft

SELECT

Publisher

IOP Publishing

Subject

Materials Chemistry,General Energy,Materials Science (miscellaneous)

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