Frustration, strain and phase co-existence in the mixed valent hexagonal iridate Ba3NaIr2O9

Author:

Garg Charu,Cervellino AntonioORCID,Nair SunilORCID

Abstract

Abstract Using detailed synchrotron diffraction, magnetization, thermodynamic and transport measurements, we investigate the relationship between the mixed valence of Ir, lattice strain and the resultant structural and magnetic ground states in the geometrically frustrated triple perovskite iridate Ba3NaIr2O9. We observe a complex interplay between lattice strain and structural phase co-existence, which is typically not observed in this family of compounds. The low temperature magnetic ground state is characterized by the absence of long-range magnetic order, and points towards the condensation of a cluster glass state from an extended regime of short range magnetic correlations.

Funder

Jawaharlal Nehru Centre for Advanced Scientific Research

Department of Science and Technology, India

Nanomission Thematic Unit Program

Publisher

IOP Publishing

Subject

Condensed Matter Physics,General Materials Science

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