DFT analysis of Re-modified WSe2 monolayers for adsorption of CO, C2H2, and C2H4

Author:

Sarkar Suman,Debnath Papiya,De Debashis,Chanda ManashORCID

Abstract

Abstract The sensing performances of the Rhenium (Re) doped Tungsten Diselenide (WSe2) monolayer for detecting small gas molecules such as carbon monoxide (CO), acetylene (C2H2), and ethylene (C2H4) have been analyzed in this paper. Density functional theory and non-equilibrium Green’s function have been used to examine the electrical and geometric structures of re-adorned WSe2 monolayer when subjected to dissolved gas analysis gases in the transformer oil. Hence, the electrochemical characteristics like Band diagram and density of states are detailed. Adsorption systems’ recovery capabilities, Mulliken population, and adsorption energy have been examined to determine their stability. Studies also show that Re-doped WSe2 monolayer exerts deformation and as a result, the band gap narrowed down. At ambient temperature (273 K–300 K), the Re-doped WSe2 exhibits better adsorption of C2H4 over C2H2 and CO as the C2H4 has higher adsorption energy compared to the C2H2 and CO. Besides, V–I characteristics of the Re doped WSe2 layer after adsorption of the CO, C2H2, and C2H4 are detailed which signifies the efficacy of the Re doped WSe2 monolayer.

Publisher

IOP Publishing

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