Evolution of the charge carrier plasmon in the one-dimensional metal TTF-TCNQ as a function of temperature and momentum

Author:

Kovbasa Nikolay,Graf LukasORCID,Knupfer MartinORCID

Abstract

Abstract We have investigated the charge carrier plasmon in the quasi one-dimensional metal TTF-TCNQ using electron energy-loss spectroscopy. Our data reveal a negative plasmon dispersion with a slope that is independent of temperature, which is in agreement to predictions from model calculations and previous room temperature data. A plasmon energy shift upon temperature is observed, and we discuss possible contributions to this shift. The spectral width of the plasmon is rather temperature independent, but increases clearly above a momentum value of about 0.3 Å−1.

Funder

Bundesministerium fuer Bildung und Forschung

Publisher

IOP Publishing

Subject

Metals and Alloys,Polymers and Plastics,Surfaces, Coatings and Films,Biomaterials,Electronic, Optical and Magnetic Materials

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