High-performance FeaTibOx catalyst loaded on ceramic filter for NOx reduction

Abstract

Abstract The FeaTibOx catalyst was loaded into the pores of porous ceramic using impregnation method for removing nitrogen oxides with selective catalytic reduction (SCR) technology. The catalytic performance over FeaTibOx catalyst was studied in detail. The Fe6Ti1Ox catalyst displayed more than 95% NOx conversion within the range of 280 °C–400 °C, and still maintained 97% NOx conversion when 300 ppm SO2 and 10 vol.% water vapor were introduced at the testing temperature of 300 °C. The influence factors (including filtration velocity, NH3/NO mole ratio and oxygen concentration) for NOx conversion over Fe6Ti1Ox catalyst were also studied. The suitable NH3/NO mole ratio and oxygen concentration was 0.9 and 6%, respectively. The XRD, N2-BET, H2-TPR, NH3-TPD and XPS were employed to investigate physicochemical property of the FeaTibOx catalyst. The results illustrated that Fe6Ti1Ox catalyst has hematite Fe2O3 and TiO2 structure, better redox properties and stronger surface acid.