Submicron drops from flapping bursting bubbles

Author:

Jiang Xinghua1ORCID,Rotily Lucas2,Villermaux Emmanuel23ORCID,Wang Xiaofei145ORCID

Affiliation:

1. Department of Environmental Science and Engineering, Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Fudan University, Shanghai 200433, China;

2. Institut de Recherche sur les Phénomènes Hors Equilibre, Aix-Marseille Université, Marseille CEDEX 13 13384, France;

3. Institut Universitaire de France, Paris 75005, France;

4. Shanghai Institute of Pollution Control and Ecological Security, Shanghai 200092, China;

5. Cluster of Interfacial Processes Against Pollution, Fudan University, Shanghai 200433, China

Abstract

Significance Bubble bursting aerosols play a critical role in forming clouds, scattering sunlight, and transporting pathogens from water to the air. Most of them are produced from the fragmentation of bubble cap film. They usually have a diameter below 1 μm. However, their physical production mechanism has remained unknown. In this work, we discovered that these drops are probably generated from flapping bubble cap film (like a flapping flag). It explains the mysterious relation between bubble size and number of drops produced per bubble, providing a fundamental framework for understanding the production flux of bubble bursting aerosols, such as sea spray aerosol, and substance transfer through the air–water interface during drop ejection.

Funder

National Natural Science Foundation of China

Natural Science Foundation of Shanghai

Publisher

Proceedings of the National Academy of Sciences

Subject

Multidisciplinary

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