Generation of intense phase-stable femtosecond hard X-ray pulse pairs

Author:

Zhang Yu1,Kroll Thomas2,Weninger Clemens34,Michine Yurina5,Fuller Franklin D.3ORCID,Zhu Diling3,Alonso-Mori Roberto3ORCID,Sokaras Dimosthenis2ORCID,Lutman Alberto A.6ORCID,Halavanau Aliaksei7,Pellegrini Claudio7ORCID,Benediktovitch Andrei8,Yabashi Makina910ORCID,Inoue Ichiro9,Inubushi Yuichi910,Osaka Taito9,Yamada Jumpei9,Babu Ganguli11,Salpekar Devashish11,Sayed Farheen N.11,Ajayan Pulickel M.11,Kern Jan12ORCID,Yano Junko12ORCID,Yachandra Vittal K.12ORCID,Yoneda Hitoki5,Rohringer Nina813,Bergmann Uwe114ORCID

Affiliation:

1. Stanford PULSE Institute, SLAC National Accelerator Laboratory, Menlo Park, CA 94025

2. Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA 94025

3. Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025

4. MAX IV Laboratory, Lund University, Lund 224 84, Sweden

5. Institute for Laser Science, The University of Electro-Communications, Chofu,Tokyo 182-8585, Japan

6. Linac & FEL Division, SLAC National Accelerator Laboratory, Menlo Park, CA 94025

7. Accelerator Research Division, SLAC National Accelerator Laboratory, Menlo Park, CA 94025

8. Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Hamburg 22607, Germany

9. RIKEN SPring-8 Center, Sayo-cho, Sayo-gun, Hyogo 679-5148, Japan

10. Japan Synchrotron Radiation Research Institute, Sayo-cho, Sayo-gun, Hyogo 679-5198, Japan

11. Department of Materials Science and NanoEngineering, Rice University, Houston, TX 77005

12. Molecular Biophysics and Integrated Bioimaging Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720

13. Department of Physics, Universität Hamburg, Hamburg 20355, Germany

14. Department of Physics, University of Wisconsin–Madison, Madison, WI 53706

Abstract

Significance The generation of phase-stable femtosecond X-ray pulse pairs will advance nonlinear spectroscopies and imaging, providing direct insight into the coupled motions of electrons and nuclei with resolution on the electronic length scale and timescale. This paper presents the generation of such pulse pairs in the X-ray domain. The approach uses X-ray free-electron laser pulses to induce highly directional, intense, phase-stable pairs of superfluorescence and seeded stimulated emission at the 5.9 keV manganese Kα 1 line. The finding is evidenced by strong interference fringes in the superfluorescence and stimulated emission signals.

Funder

DOE | Office of Science

Publisher

Proceedings of the National Academy of Sciences

Subject

Multidisciplinary

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