Command of three-dimensional solitary waves via photopatterning

Author:

Li Chao-Yi12ORCID,Tang Xing-Zhou3,Yu Xiao1,Atzin Noe3ORCID,Song Zhen-Peng2,Chen Chu-Qiao3ORCID,Abbott Nicholas L.4ORCID,Li Bing-Xiang12ORCID,de Pablo Juan J.35,Lu Yan-Qing1ORCID

Affiliation:

1. National Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing 210093, China

2. College of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology), Nanjing University of Posts and Telecommunications, Nanjing 210023, China

3. Pritzker School of Molecular Engineering, The University of Chicago, Chicago, IL 60637

4. Smith School of Chemical and Biomolecular Engineering, Cornell University, Ithaca, NY 14853

5. Center for Molecular Engineering, Argonne National Laboratory, Lemont, IL 60439

Abstract

Multidimensional solitons are prevalent in numerous research fields. In orientationally ordered soft matter system, three-dimensional director solitons exemplify the localized distortion of molecular orientation. However, their precise manipulation remains challenging due to unpredictable and uncontrolled generation. Here, we utilize preimposed programmable photopatterning in nematics to control the kinetics of director solitons. This enables both unidirectional and bidirectional generation at specific locations and times, confinement within micron-scaled patterns of diverse shapes, and directed propagation along predefined trajectories. A focused dynamical model provides insight into the origins of these solitons and aligns closely with experimental observations, underscoring the pivotal role of anchoring conditions in soliton manipulation. Our findings pave the way for diverse fundamental research avenues and promising applications, including microcargo transportation and optical information processing.

Funder

MOST | National Key Research and Development Program of China

MOST | National Natural Science Foundation of China

JST | Natural Science Foundation of Jiangsu Province

Department of Energy, Basic Energy Sciences, Division of Materials Research, Biomaterials Program

Publisher

Proceedings of the National Academy of Sciences

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