Enhanced triplet superconductivity in next-generation ultraclean UTe 2

Author:

Wu Z.1ORCID,Weinberger T. I.1ORCID,Chen J.1,Cabala A.2,Chichinadze D. V.3ORCID,Shaffer D.45,Pospíšil J.2ORCID,Prokleška J.2ORCID,Haidamak T.2ORCID,Bastien G.2,Sechovský V.2ORCID,Hickey A. J.1ORCID,Mancera-Ugarte M. J.6,Benjamin S.3,Graf D. E.3,Skourski Y.7,Lonzarich G. G.1,Vališka M.2ORCID,Grosche F. M.1ORCID,Eaton A. G.1ORCID

Affiliation:

1. Department of Physics, Cavendish Laboratory, University of Cambridge, Cambridge CB3 0HE, United Kingdom

2. Charles University, Faculty of Mathematics and Physics, Department of Condensed Matter Physics, Prague 2 121 16, Czech Republic

3. National High Magnetic Field Laboratory, Tallahassee, FL 32310

4. Department of Physics, Emory University, Atlanta, GA 30322

5. Department of Physics, University of Wisconsin-Madison, Madison, WI 53706

6. Department of Chemical Engineering and Biotechnology, University of Cambridge, Cambridge CB3 0AS, United Kingdom

7. Hochfeld-Magnetlabor Dresden, Helmholtz-Zentrum Dresden-Rossendorf, Dresden 01328, Germany

Abstract

The unconventional superconductor UTe 2 exhibits numerous signatures of spin-triplet superconductivity—a rare state of matter which could enable quantum computation protected against decoherence. UTe 2 possesses a complex phase landscape comprising two magnetic field-induced superconducting phases, a metamagnetic transition to a field-polarized state, along with pair- and charge-density wave orders. However, contradictory reports between studies performed on UTe 2 specimens of varying quality have severely impeded theoretical efforts to understand the microscopic origins of the exotic superconductivity. Here, we report a comprehensive suite of high magnetic field measurements on a generation of pristine quality UTe 2 crystals. Our experiments reveal a significantly revised high magnetic field superconducting phase diagram in the ultraclean limit, showing a pronounced sensitivity of field-induced superconductivity to the presence of crystalline disorder. We employ a Ginzburg–Landau model that excellently captures this acute dependence on sample quality. Our results suggest that in close proximity to a field–induced metamagnetic transition the enhanced role of magnetic fluctuations—that are strongly suppressed by disorder—is likely responsible for tuning UTe 2 between two distinct spin-triplet superconducting phases.

Funder

UKRI | Engineering and Physical Sciences Research Council

Gordon and Betty Moore Foundation

EC | ERC | HORIZON EUROPE European Research Council

National Science Foundation

Czech Research Infrastructures

Czech Science Foundation

Publisher

Proceedings of the National Academy of Sciences

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