Patagonian dust, Agulhas Current, and Antarctic ice-rafted debris contributions to the South Atlantic Ocean over the past 150,000 years

Author:

Barkley Anne E.1ORCID,Winckler Gisela12ORCID,Recasens Cristina1,Kaplan Michael R.1ORCID,Koffman Bess G.3ORCID,Calabozo Fernando4,Middleton Jennifer L.1ORCID,Anderson Robert F.12ORCID,Cai Yue5ORCID,Bolge Louise1,Longman Jack67ORCID,Goldstein Steven L.12ORCID

Affiliation:

1. Division of Geochemistry, Lamont-Doherty Earth Observatory of Columbia University, Palisades, NY 10964

2. Department of Earth and Environmental Sciences, Columbia University, New York, NY 10027

3. Department of Geology, Colby College, Waterville, ME 04901

4. Centro de Investigaciones en Ciencias de la Tierra, Ciudad Universitaria, Córdoba X5016CGA, Argentina

5. Nanjing Institute of Geology and Palaeontology and Center for Excellence in Life and Paleoenvironment, Chinese Academy of Sciences, Nanjing 210008, China

6. Marine Isotope Geochemistry, Institute for Chemistry and Biology of the Marine Environment, Carl von Ossietzky Universität Oldenburg, Oldenburg 26129, Germany

7. Department of Geography and Environmental Sciences, Northumbria University, Newcastle-upon-Tyne NE1 8ST, United Kingdom

Abstract

Disentangling inputs of aeolian dust, ice-rafted debris (IRD), and eroded continental detritus delivered by ocean currents to marine sediments provide important insights into Earth System processes and climate. This study uses Sr-Nd-Pb isotope ratios of the continent-derived (lithogenic) fraction in deep-sea core TN057-6 from the subantarctic Southern Ocean southwest of Africa over the past 150,000 y to identify source regions and quantify their relative contributions and fluxes utilizing a mixing model set in a Bayesian framework. The data are compared with proxies from parallel core Ocean Drilling Program Site 1090 and newly presented data from potential South America aeolian dust source areas (PSAs), allowing for an integrated investigation into atmospheric, oceanic, and cryospheric dynamics. PSA inputs varied on glacial/interglacial timescales, with southern South American sources dominating up to 88% of the lithogenic fraction (mainly Patagonia, which provided up to 68%) during cold periods, while southern African sources were more important during interglacials. During the warmer Marine Isotope Stage (MIS) 3 of the last glacial period, lithogenic fluxes were twice that of colder MIS2 and MIS4 at times, and showed unique isotope ratios best explained by Antarctic-derived IRD, likely from the Weddell Sea. The IRD intrusions contributed up to 41% at times and followed Antarctic millennial warming events that raised temperatures, causing instability of icesheet margins. High IRD was synchronous with increased bioavailable iron, nutrient utilization, high biological productivity, and decreased atmospheric CO 2 . Overall, TN057-6 sediments record systematic Southern Hemisphere climate shifts and cryospheric changes that impacted biogeochemical cycling on both glacial/interglacial and subglacial timescales.

Funder

Lamont Postdoctoral Fellowship

G. Unger Vetlesen Foundation

Swiss NSF Postdoctoral Fellowship

NSF

Storke Endowment of the Department of Earth and Environmental Sciences, Columbia University

Publisher

Proceedings of the National Academy of Sciences

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