Commensurate 4a0-period charge density modulations throughout the Bi2Sr2CaCu2O8+x pseudogap regime

Author:

Mesaros Andrej,Fujita Kazuhiro,Edkins Stephen D.,Hamidian Mohammad H.,Eisaki Hiroshi,Uchida Shin-ichi,Davis J. C. Séamus,Lawler Michael J.,Kim Eun-Ah

Abstract

Theories based upon strong real space (r-space) electron–electron interactions have long predicted that unidirectional charge density modulations (CDMs) with four-unit-cell (4a0) periodicity should occur in the hole-doped cuprate Mott insulator (MI). Experimentally, however, increasing the hole density p is reported to cause the conventionally defined wavevector QA of the CDM to evolve continuously as if driven primarily by momentum-space (k-space) effects. Here we introduce phase-resolved electronic structure visualization for determination of the cuprate CDM wavevector. Remarkably, this technique reveals a virtually doping-independent locking of the local CDM wavevector at |Q0|=2π/4a0 throughout the underdoped phase diagram of the canonical cuprate Bi2Sr2CaCu2O8. These observations have significant fundamental consequences because they are orthogonal to a k-space (Fermi-surface)–based picture of the cuprate CDMs but are consistent with strong-coupling r-space–based theories. Our findings imply that it is the latter that provides the intrinsic organizational principle for the cuprate CDM state.

Funder

U.S. Department of Energy

Simons Foundation

Engineering and Physical Sciences Research Council

Gordon and Betty Moore Foundation

Japan Ministry of Science and Education

Japan Society for the Promotion of Science

University College Cork

DOE | Brookhaven National Laboratory, Center for Emergent Superconductivity

Publisher

Proceedings of the National Academy of Sciences

Subject

Multidisciplinary

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