An atomic resolution study of a carbide phase in platinum

Author:

Witcomb M.J.,O'Keefe M.A.,Echer CJ.,Nelson C.,Turner J.H.,Dahmen U.,Westmacott K.H.

Abstract

Under normal circumstances, Pt dissolves only a very small amount of interstitial carbon in solid solution. Even so, an appropriate quench/age treatment leads to the formation of stable Pt2C {100} plate precipitates. Excess (quenched-in) vacancies play a critical role in the process by accommodating the volume and structural changes that accompany the transformation. This alloy system exhibits other interesting properties. Due to a large vacancy/carbon atom binding energy, Pt can absorb excess carbon at high temperatures in a carburizing atmosphere. In regions rich in carbon and vacancies, another carbide phase, Pt7C which undergoes an order-disorder reaction was formed. The present study of Pt carburized at 1160°C and aged at 515°C shows that other carbides in the PtxC series can be produced.

Publisher

Cambridge University Press (CUP)

Subject

General Medicine

Reference8 articles.

1. Coupled diffusion of carbon atoms and vacancies in platinum

2. Walter Somerville

3. 8. This work was supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy, under contract No. DE-AC03-76SF00098.

4. A study of precipitation in interstitial alloys—II. A new metastable carbide phase in platinum

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