14C Release in Various Chemical Forms With Gaseous Effluents From the Paks Nuclear Power Plant

Abstract

We present results of airborne 14C emission measurements from the Paks PWR nuclear power plant. Long-term release of 14C in the form of carbon dioxide or carbon monoxide and hydrocarbons were simultaneously measured. The results of internal gas-proportional and liquid scintillation counting agree well with theoretical assessments of 14C releases from pressurized water reactors. The mean value of the 14C concentration in discharged air is 130Bqm-3 and the normalized release is equal to 740GBq/GWe · yr. > 95% of 14C released is in the form of hydrocarbons, ca 4% is apportioned to CO2, and <1% to CO. Tree-ring measurements were also made and indicated a minute increase of 14C content in the vicinity of the nuclear power plant.