Contamination and Human Health Risk Assessment of Toxic Trace Elements in Drinking Water of Gilgit-Baltistan, Pakistan

Abstract

This study investigated the contamination level and risk associated with toxic trace elements in springs’ water from Gilgit-Baltistan, Pakistan. Toxic trace elements, including Hg, As, and Zn, were analyzed by metalyzer, HM 2000 serial no. MY-011-006, while elements such as Cr, Al, B, Ni, Cu, Mn, and Fe were analyzed using Metalometer HM 2000 serial no. MM005-007, the United Kingdom. The mean concentrations of TTEs in water samples from Skardu were ordered as, Mn < Cu < Fe < Zn < Al < Cr < As < Ni < Hg, in Gilgit, Mn < Cu < Zn < Ni < B < Cr < Fe < As < Hg, in Ghizer Cu < Mn < Zn < Ni < Cr < Fe < As < Hg, while in Nagar the concentration of TTEs in water samples were ordered as Cu < Mn < Fe < Ni < Al < Cr < Zn < As < Hg. Results obtained from this study showed that the concentrations of As, Hg, Ni, Cr, Al, and Mn in some water samples were higher than the limits recommended by WHO and Pak-NDWQS. However, the chronic daily intake indices (CDIs) and health risk index (HRI) in all samples were found below the US-EPA standards. The correlation analysis revealed a positive association among different elements, which revealed that the sources of TTES in water samples were mainly geological strata and anthropogenic activities.