Understanding the Mechanistic Role of Lithium in Accelerated Corrosion of Zirconium Alloys Using Advanced Characterization and Atomistic Simulation

Author:

Garner Alistair12,Gillen Conor1ORCID,Stephens Gareth3ORCID,Styman Paul4,Armson Sam1ORCID,Robinson Jacqueline1,Liu Junliang5ORCID,Carruthers Alexander2,Pickering Felicity1ORCID,Sherry Sarah1,Chan ChoenMay1,Fenwick Mark1,Hulme Helen1,Ortner Susan4,Riley Chris6,Grovenor Chris5,Frankel Philipp2,Middleburgh Simon C.3ORCID,Cole-Baker Aidan1

Affiliation:

1. Jacobs, Walton House, Birchwood Park, Warrington, WA3 6GA, GB

2. Dept. of Materials, University of Manchester, Oxford Rd., M13 9PL, GB

3. Nuclear Futures Institute, Bangor University, Bangor, LL57 1UT, GB

4. National Nuclear Laboratory, Culham Science Centre, Abingdon, OX14 3DB, GB

5. Dept. of Materials, University of Oxford, Parks Rd., OX1 3PH, GB

6. Rolls-Royce, Raynesway, Derby, DE21 7BE, GB

Publisher

ASTM International

Reference49 articles.

1. F. Nordmann, “PWR and BWR Chemistry Optimization,” Nuclear Engineering International Magazine, (December 2011): 24–29.

2. D. Schrire, P. Gabrielsson, M. Hemlin, K. Carling, H. Nylén, F. Ehrlén, K. Johnson et al., “Corrosion Hydrogen and Lithium Pickup of Optimized ZIRLO Cladding Operated at High Duty with High Lithium Levels” (paper presentation, TopFuel 2021, Santander, Spain, October 24–28, 2021).

3. F. Garzarolli, J. Pohlmeyer, S. Trapp-Pritsching, and H. G. Weidinger, “Influence of Various Additions to Water on Zircaloy-4 Corrosion in Autoclave Tests at 350°C,” in Proceedings of the IAEA Technical Committee Meeting on Fundamental Aspects of Corrosion of Zr-Alloys in Water Reactor Environments (Vienna, Austria: International Atomic Energy Agency, 1990), 65–72.

4. I. L. Bramwell, P. D. Parsons, and D. Tice, “Corrosion of Zircaloy-4 PWR Fuel Cladding in Lithiated and Borated Water Environments,” in Zirconium in the Nuclear Industry: 9th International Symposium, ed. C. M. Eucken and A. M. Garde (West Conshohocken, PA: ASTM International, 1991), 628–642, https://doi.org/10.1520/STP25532S

5. D. Pêcheur, J. Godlewski, J. Peybernès, L. Fayette, M. Noé, A. Frichet, and O. Kerrec, “Contribution to the Understanding of the Effect of the Water Chemistry on the Oxidation Kinetics of Zircaloy-4 Cladding,” in Zirconium in the Nuclear Industry: 12th International Symposium, ed. G. P. Sabol and G. D. Moan (West Conshohocken, PA: ASTM International, 2000), 793–811, https://doi.org/10.1520/STP14328S

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