Heteropolyacid-loaded MOF-derived mesoporous zirconia catalyst for chemical degradation of rhodamine B

Author:

Wang Jialu1,Yu Rongfei1,Li Zhenying1,Yang Fen1,Luo Linmin1,Wang Dandan1,Cheng Huan1,Zhang Yutao1,Zhang Qiuyun1

Affiliation:

1. College Rural Revitalization Research Center of Guizhou, School of Resource and Environmental Engineering, Engineering Technology Center of Control and Remediation of Soil Contamination of Guizhou Science and Technology Department, Anshun University , 561000 , Guizhou , China

Abstract

Abstract In this article, silicotungstic acid (STA)-loaded metal–organic framework (MOF)-derived composites (C-STA@ZrO2) were successfully synthesized by simple strategies. X-ray diffraction, Fourier transform infrared, scanning electron microscopy, energy-dispersive X-ray, N2 physisorption, UV-vis diffuse reflection spectroscopy, and X-ray photoelectron spectroscopy techniques were used to characterize the as-obtained composites. Intriguingly, C-STA@ZrO2 exhibits excellent photocatalytic performance, and rhodamine B (RhB) (40 mg·L−1) in water can be degraded to 93.9% after 120 min of irradiation. Moreover, various catalysts, catalyst dosage, and dye concentrations on RhB degradation were evaluated. Besides, the reusability of C-STA@ZrO2 was also investigated. This work may provide a new and significant guideline for exploring excellent performance of MOF-derived hybrid material for wastewater purification.

Publisher

Walter de Gruyter GmbH

Subject

Health, Toxicology and Mutagenesis,Industrial and Manufacturing Engineering,Fuel Technology,Renewable Energy, Sustainability and the Environment,General Chemical Engineering,Environmental Chemistry

Cited by 1 articles. 订阅此论文施引文献 订阅此论文施引文献,注册后可以免费订阅5篇论文的施引文献,订阅后可以查看论文全部施引文献

1. Use and applications of metal-organic frameworks (MOF) in dye adsorption: Review;Journal of Environmental Chemical Engineering;2023-10

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