Simultaneous removal efficiency of H2S and CO2 by high-gravity rotating packed bed: Experiments and simulation

Author:

Tran Lien Thi12,Le Tuan Minh12,Nguyen Tuan Minh1,Tran Quoc Toan23,Le Xuan Duy3,Pham Minh Quan23,Lam Van Tan45,Van Do Manh12

Affiliation:

1. Institute of Environmental Technology, Vietnam Academy of Science and Technology , 18 Hoang Quoc Viet, Cau Giay , Hanoi , 100000 , Vietnam

2. Graduate University of Science and Technology, Vietnam Academy of Science and Technology , 18 Hoang Quoc Viet, Cau Giay , Hanoi , 100000 , Vietnam

3. Institute of Natural Products Chemistry, Vietnam Academy of Science and Technology , 18 Hoang Quoc Viet, Cau Giay , Hanoi , 100000 , Vietnam

4. NTT Hi-Tech Institute, Nguyen Tat Thanh University , Ho Chi Minh City , 755414 , Vietnam

5. Center of Excellence for Green Energy and Environmental Nanomaterials, Nguyen Tat Thanh University , Ho Chi Minh City , Vietnam

Abstract

Abstract This study explores the possibility of applying high-gravity rotating packed bed (HGRPB) in removing H2S and CO2 from biogas. Ca(OH)2 aqueous solution was used as the absorbent in this study. Different experimental conditions including solution pH, rotating speed (R S) of HGRPB, gas flow rate (Q G), and liquid flow rate (Q L) were investigated with respect to the removal efficiency (E) of H2S and CO2. The experimental and simulated results show that the optimal removal efficiency of H2S and CO2 using HGRPB achieved nearly the same as 99.38 and 99.56% for removal efficiency of H2S and 77.28 and 77.86% for removal efficiency of CO2, respectively. Such efficiencies corresponded with the following optimal conditions: a solution pH of 12.26, HGRPB reactor with the rotating speed of 1,200 rpm, the gas flow rate of 2.46 (L/min), and the liquid flow rate of 0.134 (L/min).

Publisher

Walter de Gruyter GmbH

Subject

Materials Chemistry,General Chemistry

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