Tunable high-order harmonic generation in GeSbTe nano-films

Author:

Korolev Viacheslav1,Sinelnik Artem D.1ORCID,Rybin Mikhail V.23,Lazarenko Petr4,Kushchenko Olga M.2ORCID,Glukhenkaya Victoria4,Kozyukhin Sergey5ORCID,Zuerch Michael16,Spielmann Christian1,Pertsch Thomas178ORCID,Staude Isabelle1,Kartashov Daniil1ORCID

Affiliation:

1. 9378 Friedrich-Schiller University Jena , Jena , Germany

2. 65071 ITMO University , St. Petersburg , Russia

3. Ioffe Institute , St. Petersburg , Russia

4. 386236 National Research University of Electronic Technology , Moscow , Russia

5. 201631 N.S. Kurnakov Institute of General and Inorganic Chemistry , Moscow , Russia

6. University of California at Berkeley , Berkeley , USA

7. Fraunhofer-Institute for Applied Optics and Precision Engineering IOF , Jena , Germany

8. Max Planck School of Photonics , Jena , Germany

Abstract

Abstract High-order harmonic generation (HHG) in solids opens new frontiers in ultrafast spectroscopy of carrier and field dynamics in condensed matter, picometer resolution structural lattice characterization and designing compact platforms for attosecond pulse sources. Nanoscale structuring of solid surfaces provides a powerful tool for controlling the spatial characteristics and efficiency of the harmonic emission. Here we study HHG in a prototypical phase-change material Ge2Sb2Te5 (GST). In this material the crystal phase can be reversibly changed between a crystalline and amorphous phase by light or electric current mediated methods. We show that optical phase-switching is fully reversible and allows for dynamic control of harmonic emission. This introduces GST as new addition to materials that enable flexible metasurfaces and photonic structures that can be integrated in devices and allow for ultrafast optical control.

Funder

Bundesministerium für Bildung und Forschung

European Union’s Horizon 2020

German Research Foundation DFG under Collaborative Research Center SFB 1375 “NOA”

Russian Science Foundation

Carl Zeiss Foundation

Publisher

Walter de Gruyter GmbH

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