X-ray absorption spectroscopy investigations on radioactive matter using MARS beamline at SOLEIL synchrotron-Reference-Cited by-同舟云学术

X-ray absorption spectroscopy investigations on radioactive matter using MARS beamline at SOLEIL synchrotron

Published:2014-05-19 Issue:11 Volume:102 Page:957-972
ISSN:0033-8230
Container-title:Radiochimica Acta
language:en
Short-container-title:

Author:

LLorens Isabelle¹,Solari Pier Lorenzo¹,Sitaud Bruno¹,Bes René,Cammelli Sebastiano¹,Hermange Hervé¹,Othmane Guillaume²,Safi Sami³,Moisy Philippe⁴,Wahu Sandrine⁵,Bresson Carole⁶,Schlegel Michel L.⁶,Menut Denis⁷,Bechade Jean-Luc⁷,Martin Philippe⁸,Hazemann Jean-Louis⁹,Proux Olivier¹⁰,Den Auwer Christophe¹¹

Affiliation:

1. Synchrotron SOLEIL,Ligne de lumière MARS, L'Orme des Merisiers, Saint Aubin, BP 48, F-91192 Gif-sur-Yvette Cedex, France

2. Institut de Minéralogie et de Physique des Milieux Condensés, UMR 7590 CNRS-Université Pierre et Marie Curie/Paris VI-IRD 4 Place Jussieu, F-75252 Paris Cedex 05, France

3. Institut de Physique Nucléaire d'Orsay, UMR8608 CNRS-Université Paris-Sud XI Orsay, 15 Rue Georges Clémenceau, F-91406 Orsay Cedex, France

4. CEA, Nuclear Energy Division, RadioChemistry and Process Department, F-30207 Bagnols sur Ceze, France

5. CEA saclay, DEN/DPC/SECR, F91191 Gif-sur-Yvette Cedex, France

6. CEA saclay, DEN/DPC/SEARS, F91191 Gif-sur-Yvette Cedex, France

7. CEA, DEN, Service de Recherches Métallurgiques Appliquées, F-91191 Gif-sur-Yvette Cedex, France

8. CEA, DEN, DEC, F-13108 Saint Paul Lez Durance Cedex, France

9. Institut Néel, UPR 2940 CNRS, F-38042 Grenoble Cedex 9, France

10. Observatoire des Sciences de l'Univers de Grenoble, UMS 832 CNRS Université Joseph Fourier, F-38041 Grenoble Cedex 9, France

11. Institut de Chimie de Nice, UMR7272 CNRS-Université de Nice Sophia Antipolis, Campus Valrose, 28 Avenue Valrose, F-06108 Nice Cedex 2, France

Abstract

Abstract The MARS beamline at the SOLEIL synchrotron is dedicated to the characterization of radioactive material samples. One great advantage of the beamline is the possibility to characterize about 380 radionuclides by different X-ray techniques in the same place. This facility is unique in Europe. A wide energy range from around 3.5 keV to 36 keV K-edges from K to Cs, and L3 edges from Cd to Am and beyond can be used. The MARS beamline is optimized for X-ray absorption spectroscopy techniques (XANES/EXAFS), powder diffraction (XRD) but x-ray fluorescence (XRF) analysis, High Energy Resolution Fluorescence Detected -XAS (HERFD-XAS), X-ray Emission (XES) and μ-XAS/XRD are also possible. A description of the beamline as well as its performances are given in a first part. Then some scientific examples of XAS studies from users are presented which cover a wide variety of topics in radiochemistry and nuclear materials.

Publisher

Walter de Gruyter GmbH

Subject

Physical and Theoretical Chemistry

Link

https://www.degruyter.com/document/doi/10.1515/ract-2013-2241/pdf

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