Measurement of 197Au(n,γ)198gAu reaction cross-section at the neutron energies of 1.12, 2.12, 3.12 and 4.12 MeV

Author:

Vansola Vibha1,Ghosh Reetuparna2,Badwar Sylvia2,Lawriniang Bioletty Mary2,Gopalakrishna Arjun3,Naik Haladhara4,Naik Yeshwant5,Tawade Nilesh Subhash4,Sharma Suresh Chand6,Bhatt Jignesh Pravinchandra7,Gupta Shri Krishna7,Sarode Shankar7,Mukherjee Surjit1,Singh Nand Lal1,Singh Pitambar7,Goswami Ashok4

Affiliation:

1. Department of Physics, Faculty of Science, M. S. University, Baroda-390002, India

2. Department of Physics, North Eastern Hill University, Shillong, Meghalaya-793022, India

3. Medical Cyclotron Facility, Board of Radiation and Isotope Technology, Radiation Medicine Centre, Mumbai-400012, India

4. Radiochemistry Division, Bhabha Atomic Research Centre, Mumbai-400085, India

5. Product Development Division, Bhabha Atomic Research Centre, Mumbai-400085, India

6. Nuclear Physics Division, Bhabha Atomic Research Centre, Mumbai-400085, India

7. Ion Accelerator Development Division, Bhabha Atomic Research Centre, Mumbai-400085, India

Abstract

Abstract The 197Au(n, γ)198Au reaction cross-sections at the neutron energies of 1.12, 2.12, 3.12 and 4.12 MeV were determined by using activation and off-line γ-ray spectrometric technique. The mono-energetic neutron energies of 1.12–4.12 MeV were generated from the 7Li(p, n) reaction by using the proton energies of 3 and 4 MeV from the folded tandem ion beam accelerator (FOTIA) at BARC as well as 5 and 6 MeV from the Pelletron facility at TIFR, Mumbai. The 115In(n,γ)116mIn reaction cross-section was used as the neutron flux monitor. The 197Au(n, γ)198Au reaction cross-section at the neutron energies of 3.12 and 4.12 MeV are reported for the first time. The 197Au(n, γ)198Au reaction cross-sections at 1.12 and 2.12 MeV are close to the literature data of in between neutron energies. The 197Au(n, γ)198Au cross-section was also calculated theoretically by using the computer code TALYS 1.6 and found to be higher than the experimental data of present work and literature data within the neutron energies of 0.8 to 4 MeV.

Publisher

Walter de Gruyter GmbH

Subject

Physical and Theoretical Chemistry

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