Integral measurement of spectrum-averaged cross sections of a few threshold reactions induced by fast neutrons of a TRIGA reactor: comparison with integrated data from excitation functions given in various data libraries

Author:

Uddin Md. Shuza1,Rafee K. A.2,Hossain S. M.1,Khan R.1,Qaim S. M.3

Affiliation:

1. Institute of Nuclear Science and Technology (INST), Atomic Energy Research Establishment , Savar, GPO Box-3787 , Dhaka-1000 , Bangladesh

2. Department of Nuclear Engineering , University of Dhaka , Dhaka , Bangladesh

3. Institut für Neurowissenschaften und Medizin, INM-5: Nuklearchemie, Forschungszentrum Jülich , D-52425 Jülich , Germany

Abstract

Abstract Integral cross sections of the reactions 24Mg(n,p)24Na, 27Al(n,p)27Mg, 27Al(n,α)24Na, 58Ni(n,d + np)57Co and 60Ni(n,p)60Co were measured for the first time using the fast neutron spectrum of a TRIGA reactor extending from 0.5 to 20 MeV. The values obtained in this work were comparable with the recommended values for a pure 235U prompt fission spectrum. The measured integral value was utilized for integral test of excitation function of each reaction given in some data libraries, namely ENDF/B-VIII.0, TENDL-2017, IRDFF-1.05 and ROSFOND-2010. The integral measurements are generally consistent with the integrated values within 5 %, except for a few cases, e. g. the reaction 60Ni(n,p)60Co, where the data libraries appear to need improvement.

Publisher

Walter de Gruyter GmbH

Subject

Physical and Theoretical Chemistry

Reference22 articles.

1. Uddin, M. S., Sudár, S., Hossain, S. M., Khan, R., Zulquarnain, M. A., Qaim, S. M.: Fast neutron spectrum unfolding of a TRIGA Mark II reactor and measurement of spectrum-averaged cross sections: integral tests of differential cross sections of neutron threshold reactions. Radiochim. Acta 101, 613 (2013).

2. Uddin, M. S., Zaman, M. R., Hossain, S. M., Qaim, S. M.: Radiochemical measurement of neutron–spectrum averaged cross sections for the formation of 64Cu and 67Cu via the (n,p) reaction at a TRIGA Mark-II reactor: feasibility of simultaneous production of the theragnostic pair 64Cu/67Cu. Radiochim. Acta 102, 473 (2014).

3. IRDFF-1.05 (The International Reactor Dosimetry File), IAEA, Vienna, available at: https://www-nds.iaea.org/IRDFF/ (2014).

4. Koning, A. J., Rochman, D.: TENDL-2017, TALYS-based Evaluated Nuclear Data Library, Release date: December 30, 2017, available at: https://tendl.web.psi.ch/tendl_2017/tendl2017.html.

5. ENDF/B-VIII.0: National Nuclear Data Center, Brookhaven National Laboratory, USA, Database version of 20 December 2018, available at: https://www.nndc.bnl.gov/endf/ (2018).

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