Gamma-spectrometric measurement procedure for a clearance concept of radioactively contaminated mercury from nuclear facilities

Author:

Klaß LarissaORCID,Ritz Philipp,Hirsch Marius,Kettler John,Havenith Andreas,Wilden AndreasORCID,Modolo GiuseppeORCID

Abstract

AbstractRadioactive mercury waste constitutes a significant challenge, as no approved disposal concept yet exists for such waste in Germany. This work describes a decontamination and measurement procedure for a possible clearance of mercury from nuclear facilities and release into reuse or conventional hazardous waste disposal to reduce the amount of mercury in a nuclear repository. The measurement setup and procedure were developed and evaluated including Monte-Carlo N-Particle® Transport Code (MCNP® and Monte Carlo N-Particle® are registered trademarks owned by Los Alamos National Security, LLC, manager and operator of Los Alamos National Laboratory, (Werner 2018, Werner 2017)), simulations to ensure conservative assumptions during the measurements. Results from decontaminated mercury samples show that a clearance pursuant to the German regulations would be feasible.

Funder

Bundesministerium für Bildung und Forschung

Forschungszentrum Jülich GmbH

Publisher

Springer Science and Business Media LLC

Subject

Health, Toxicology and Mutagenesis,Public Health, Environmental and Occupational Health,Spectroscopy,Pollution,Radiology, Nuclear Medicine and imaging,Nuclear Energy and Engineering,Analytical Chemistry

Reference44 articles.

1. Werner CJ et al. (2018) MCNP 6.2 Release Notes. Report LA-UR-18–20808, Los Alamos National Laboratory, Los Alamos, Indiana

2. Werner (editor) CJ (2017) MCNP Users Manual—code version 6.2. Report LA-UR-17–29981, Los Alamos National Laboratory, Los Alamos, Indiana

3. Management of Problematic Waste and Material Generated During the Decommissioning of Nuclear Facilities (2006) Technical Reports Series 441. International Atomic Energy Agency (IAEA), Vienna, Austria

4. Shcherbina N, Klaß L, Deissmann G, Bosbach D (2017) Research for the safe management of nuclear wastes: The special case of 'problematic' radioactive waste streams. In: Bruhns H

5. (ed) Frühjahrstagung des Arbeitskreises Energie in der Deutschen Physikalischen Gesellschaft, Münster, 27-29 March 2017 2017. Arbeitskreis Energie (AKE) in der DPG, Bad Honnef, pp 121-134

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