Fabrication and performance of atmospheric plasma sprayed solid oxide fuel cells with liquid antimony anodes

Author:

Jiang Yidong,Mo Wenfei,Cao Tianyu,Shi YixiangORCID,Cai Ningsheng

Abstract

AbstractA solid oxide fuel cell (SOFC) with a liquid antimony anode (LAA) is a potential energy conversion technology for the use of impurity-containing fuels. Atmospheric plasma spraying (APS) technology has become a promising LAA-SOFC preparation method because of its economy and convenience. In this paper, button SOFCs with different cathode materials and ratios of pore former were prepared by the APS method and were operated at 750 °C. The effect of the cathode structure on the electrochemical performance of the LAA-SOFCs was analyzed, and an optimized spraying method for LAA-SOFCs was developed. A tubular LAA-SOFC was prepared using the APS method based on the optimized spraying method, and a peak power of 2.5 W was reached. The tubular cell was also measured at a constant current of 2 A for 20 h and was fed with a sulfur-containing fuel to demonstrate its impurity resistance and electrode stability.

Funder

the National Key R&D Program of China

the Huaneng Group Science and Technology Research Project

the Beijing Natural Science Foundation Outstanding Youth Science Foundation Project

the National High Level Talents Special Support Plan

the Tsinghua University Initiative Scientific Research Program

Publisher

Springer Science and Business Media LLC

Subject

Energy Engineering and Power Technology,Geotechnical Engineering and Engineering Geology

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