SYNTHESIS AND CHARACTERIZATION OF A RODLIKE LIQUID CRYSTALLINE POLYURETHANE OLIGOMER

Author:

WEI CHUN1,GAO QIU-SHAN1,GONG YONG-YANG1,XIONG XUE-MEI1,SHEN XIN1

Affiliation:

1. Key Laboratory of New Processing Technology for Nonferrous Metals and Materials, Ministry of Education, Guilin University of Technology, Guilin 541004, P. R. China

Abstract

A novel rodlike liquid crystalline polyurethane (LCPU) oligomer was synthesized by polyaddition of hexane-1,6-diylbis(4-hydroxybenzoate) with toluene 2,4-diissocyanate in N, N′-dimethylformamide solution. The properties of the LCPU oligomer were investigated by FT-IR, DSC, TGA, POM, WAXD and SEM. The LCPU oligomer was a yellow powder at room temperature, which maintained a stable rodlike microstructure below its melting point, and had high crystallinity. The LCPU oligomer exhibited thermotropic liquid crystalline properties between 166–183°C, and the smectic-A phase with focal conic fan textures at the liquid crystal state was observed by POM. The decomposition temperature of the LCPU oligomer at 5% weight loss was 282°C.

Publisher

World Scientific Pub Co Pte Lt

Subject

General Materials Science

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