Estimating 2010–2015 anthropogenic and natural methane emissions in Canada using ECCC surface and GOSAT satellite observations
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Published:2021-12-13
Issue:23
Volume:21
Page:18101-18121
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ISSN:1680-7324
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Container-title:Atmospheric Chemistry and Physics
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language:en
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Short-container-title:Atmos. Chem. Phys.
Author:
Baray Sabour, Jacob Daniel J., Maasakkers Joannes D.ORCID, Sheng Jian-XiongORCID, Sulprizio Melissa P., Jones Dylan B. A., Bloom A. Anthony, McLaren RobertORCID
Abstract
Abstract. Methane emissions in Canada have both anthropogenic and
natural sources. Anthropogenic emissions are estimated to be 4.1 Tg a−1
from 2010–2015 in the National Inventory Report submitted to the United
Nation's Framework Convention on Climate Change (UNFCCC). Natural emissions,
which are mostly due to boreal wetlands, are the largest methane source in
Canada and highly uncertain, on the order of ∼ 20 Tg a−1
in biosphere process models. Aircraft studies over the last several years
have provided “snapshot” emissions that conflict with inventory estimates.
Here we use surface data from the Environment and Climate Change Canada
(ECCC) in situ network and space-borne data from the Greenhouse Gases
Observing Satellite (GOSAT) to determine 2010–2015 anthropogenic and
natural methane emissions in Canada in a Bayesian inverse modelling
framework. We use GEOS-Chem to simulate anthropogenic emissions comparable
to the National Inventory and wetlands emissions using an ensemble of
WetCHARTS v1.0 scenarios in addition to other minor natural sources. We
conduct a comparative analysis of the monthly natural emissions and yearly
anthropogenic emissions optimized by surface and satellite data
independently. Mean 2010–2015 posterior emissions using ECCC surface data
are 6.0 ± 0.4 Tg a−1 for total anthropogenic and 11.6 ± 1.2 Tg a−1 for total natural emissions. These results agree with our
posterior emissions of 6.5 ± 0.7 Tg a−1 for total
anthropogenic and 11.7 ± 1.2 Tg a−1 for total natural emissions using GOSAT data.
The seasonal pattern of posterior natural emissions using either dataset
shows slower to start emissions in the spring and a less intense peak in
the summer compared to the mean of WetCHARTS scenarios. We combine ECCC and
GOSAT data to characterize limitations towards sectoral and provincial-level
inversions. We estimate energy + agriculture emissions to be 5.1 ± 1.0 Tg a−1, which is 59 % higher than the national inventory. We
attribute 39 % higher anthropogenic emissions to Western Canada than the
prior. Natural emissions are lower across Canada. Inversion results are
verified against independent aircraft data and surface data, which show
better agreement with posterior emissions. This study shows a readjustment
of the Canadian methane budget is necessary to better match atmospheric
observations with lower natural emissions partially offset by higher
anthropogenic emissions.
Funder
Natural Sciences and Engineering Research Council of Canada
Publisher
Copernicus GmbH
Subject
Atmospheric Science
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