Impact of hybrid surfaces on the droplet breakup dynamics in microgravity slug flow: A dynamic contact angle analysis

Abstract

Microfluidic devices, which enable precise control and manipulation of fluids at the microscale, have revolutionized various fields, including chemical synthesis and space technology. A comprehensive understanding of fluid behavior under diverse conditions, particularly in microgravity, is essential for optimizing the design and performance of these devices. This paper aims to investigate the effects of discontinuous wettability on droplet breakup structures under microgravity conditions using a microchannel wall. The approach we adopt is underpinned by the volume-of-fluid methodology, an efficient technique renowned for its accurate resolution of the fluid interface in a two-phase flow. Furthermore, a modified dynamic contact angle model is employed to precisely predict the shape of the droplet interface at and near the wall. Our comprehensive model considers influential parameters such as slug length and droplet generation frequency, thereby providing crucial insights into their impact on the two-phase interface velocity. Validated against existing literature data, our model explores the impact of various configurations of discontinuous wettability on breakup morphology. Our findings highlight the significance of employing a dynamic contact angle methodology for making accurate predictions of droplet shape, which is influenced by the wall contact angle. Emphasis is placed particularly on the effects of slug length and droplet generation frequency. Notably, we demonstrate that the use of a hybrid surface at the junction section allows for precise control over the shape and size of the daughter droplets, contrasting with the symmetrical division observed on uniformly hydrophilic or superhydrophobic surfaces. This study contributes valuable insights into the complex dynamics of the droplet breakup process, which has profound implications for the design and optimization of microfluidic devices operating under microgravity conditions. Such insights are further poised to augment applications in space exploration, microreactors, and more.