Anionic aza 8π-electrocyclization as an unprecedented pathway versus 7-endo-dig: DFT study on the mechanism of base-catalyzed benzofuroazepine synthesis via cyclization of (2-alkynylbenzyl)oxy nitriles-Reference-Cited by-同舟云学术

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Anionic aza 8π-electrocyclization as an unprecedented pathway versus 7-endo-dig: DFT study on the mechanism of base-catalyzed benzofuroazepine synthesis via cyclization of (2-alkynylbenzyl)oxy nitriles

Published:2024 Issue: Volume: Page:
ISSN:1463-9076
Container-title:Physical Chemistry Chemical Physics
language:en
Short-container-title:Phys. Chem. Chem. Phys.

Author:

Amiri Omid¹,Bazgir Ayoob¹^ORCID

Affiliation:

1. Department of Organic Chemistry, Shahid Beheshti University, Tehran 1983969411, Iran

Abstract

DFT calculations are used to disclose the mechanism of Brønsted base-mediated cyclization of 2-alkynylbenzyloxy nitriles for the synthesis of benzofuroazepines.

Funder

Shahid Beheshti University

Iran National Science Foundation

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/CP/D4CP02458C

Reference36 articles.

1. Syntheses of the Stemona Alkaloids (±)-Stenine, (±)-Neostenine, and (±)-13-Epineostenine Using a Stereodivergent Diels–Alder/Azido-Schmidt Reaction

2. Recent advances in 8π electrocyclization reactions

3. Stereocontrolled Synthesis of (−)-Galanthamine

4. Allenamide‐Initiated Cascade [2+2+2] Annulation Enabling the Divergent Total Synthesis of (−)‐Deoxoapodine, (−)‐Kopsifoline D and (±)‐Melotenine A

5. Biomimetic diversity-oriented synthesis of benzannulated medium rings via ring expansion

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