Achieving 17.5% efficiency for polymer solar cells via a donor and acceptor layered optimization strategy

Author:

Xu Wenjing1,Li Xiong2ORCID,Jeong Sang Young3,Son Jae Hoon3,Zhou Zhengji4ORCID,Jiang Qiuju5,Woo Han Young3ORCID,Wu Qinghe5ORCID,Zhu Xixiang1,Ma Xiaoling1,Zhang Fujun1ORCID

Affiliation:

1. Key Laboratory of Luminescence and Optical Information, Ministry of Education, Beijing Jiaotong University, 100044, Beijing, China

2. Department of Physics, Beijing Technology and Business University, 100048, Beijing, China

3. Organic Optoelectronic Materials Laboratory, Department of Chemistry, College of Science, Korea University, 02841, Seoul, Republic of Korea

4. Key Lab for Special Functional Materials, Ministry of Education, National and Local Joint Engineering Research Center for High-Efficiency Display and Lighting Technology, and School of Materials, Henan University, 475004, Kaifeng, Henan Province, China

5. Department of Chemistry and Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong, Shantou University, 515063, Guangdong, China

Abstract

PCEs of 14.81% and 17.53% are achieved in BHJ and LbL-PSCs with PNTB6-Cl and Y6 as active layers, and DPE and DFB as solvent additives, respectively. The PCE improvement can be confirmed from the optimized crystallinity and morphology of films.

Funder

National Natural Science Foundation of China

China Postdoctoral Science Foundation

Beijing Municipal Natural Science Foundation

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,General Chemistry

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