Efficient and chemoselective imine synthesis catalyzed by a well-defined PN3-manganese(ii) pincer system

Author:

Gholap Sandeep Suryabhan1ORCID,Dakhil Abdullah Al12,Chakraborty Priyanka1,Dighe Shashikant3,Rahman Mohammad Misbahur1,Dutta Indranil1ORCID,Hengne Amol3,Huang Kuo-Wei13ORCID

Affiliation:

1. KAUST Catalysis Center and Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology, Thuwal 23955-6900, Saudi Arabia

2. Department of Chemistry, College of Science, Imam Mohammad Ibn Saud Islamic University, Riyadh 11432-5701, Saudi Arabia

3. Agency for Science, Technology and Research, Institute of Materials Research and Engineering and Institute of Sustainability for Chemicals, Energy and Environment, Singapore

Abstract

The highly efficient reductive amination of aldehydes with ammonia (NH3) and hydrogen (H2) to form secondary imines is described, as well as the dehydrogenative homocoupling of benzyl amines.

Funder

King Abdullah University of Science and Technology

Publisher

Royal Society of Chemistry (RSC)

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