Unraveling the complexity of atmospheric brown carbon produced by smoldering boreal peat using size-exclusion chromatography with selective mobile phases

Author:

Lyu Ming1234ORCID,Thompson Dan K.534ORCID,Zhang Nianci1234ORCID,Cuss Chad W.67234ORCID,Young Cora J.1894ORCID,Styler Sarah A.123410ORCID

Affiliation:

1. Department of Chemistry

2. University of Alberta

3. Edmonton

4. Canada

5. Natural Resources Canada – Northern Forestry Centre

6. SWAMP Lab

7. Department of Renewable Resources

8. York University

9. Toronto

10. Department of Chemistry & Chemical Biology

Abstract

Water-soluble BrC in freshly emitted boreal peat combustion particulate matter spans a wide range of molecular sizes, polarities, and light absorption properties; in addition, its largest fraction undergoes solvent-dependent aggregation/dissociation.

Funder

Natural Sciences and Engineering Research Council of Canada

Mitacs

Canada Foundation for Innovation

Canada Research Chairs

University of Alberta

Publisher

Royal Society of Chemistry (RSC)

Reference77 articles.

1. A technology-based global inventory of black and organic carbon emissions from combustion

2. Global fire emissions and the contribution of deforestation, savanna, forest, agricultural, and peat fires (1997–2009)

3. IPCC , Climate Change 2013: The Physical Science Basis. Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change , ed. T. F. Stocker , D. Qin , G.-K. Plattner , M. Tignor , S. K. Allen , J. Boschung , A. Nauels , Y. Xia , V. Bex and P. M. Midgley , Cambridge University Press , Cambridge, United Kingdom and New York, NY, USA , 2013 , pp. 1535

4. Lifecycle of light-absorbing carbonaceous aerosols in the atmosphere

5. Bounding the role of black carbon in the climate system: A scientific assessment

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