Entropy driven chain effects on ligation chemistry-Reference-Cited by-同舟云学术

Entropy driven chain effects on ligation chemistry

Published:2015 Issue:2 Volume:6 Page:1061-1074
ISSN:2041-6520
Container-title:Chemical Science
language:en
Short-container-title:Chem. Sci.

Author:

Pahnke Kai¹²³⁴⁵,Brandt Josef⁶⁷⁵⁸⁹,Gryn'ova Ganna¹⁰¹¹¹²¹³¹⁴,Lindner Peter¹⁵¹⁶¹⁷,Schweins Ralf¹⁵¹⁶¹⁷,Schmidt Friedrich Georg¹⁸¹⁹⁵,Lederer Albena⁶⁷⁵⁸⁹,Coote Michelle L.¹⁰¹¹¹²¹³¹⁴,Barner-Kowollik Christopher¹²³⁴⁵

Affiliation:

1. Preparative Macromolecular Chemistry

2. Institut für Technische Chemie und Polymerchemie

3. Karlsruhe Institute of Technology (KIT)

4. 76131 Karlsruhe

5. Germany

6. Leibniz-Institut für Polymerforschung Dresden

7. 01069 Dresden

8. Technische Universität Dresden

9. 01062 Dresden

10. ARC Centre of Excellence for Electromaterials Science

11. Research School of Chemistry

12. Australian National University

13. Canberra

14. Australia

15. Institut Laue-Langevin (ILL)

16. 38042 Grenoble CEDEX 9

17. France

18. Evonik Industries AG

19. 45764 Marl

Abstract

Entropic chain effects on dynamic bonding reactions are shown to enable the tuning of reaction equilibria not only by changing the mass of the reactants, but also by merely altering the building block side chain structure and thus the intrinsic stiffness. The findings enable a step change for the design of on-demand bonding systems and reversible ligation chemistry in general.

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2015/SC/C4SC02908A

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