Polyenolate-mediated reaction cascade initiated by higher-order-cycloaddition for the construction of polycarbocyclic scaffolds-Reference-Cited by-同舟云学术

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Polyenolate-mediated reaction cascade initiated by higher-order-cycloaddition for the construction of polycarbocyclic scaffolds

Published:2024 Issue:6 Volume:11 Page:1700-1705
ISSN:2052-4129
Container-title:Organic Chemistry Frontiers
language:en
Short-container-title:Org. Chem. Front.

Author:

Cieśliński Adam¹,Skrzyńska Anna¹,Przydacz Artur¹,Albrecht Łukasz¹^ORCID

Affiliation:

1. Institute of Organic Chemistry, Faculty of Chemistry, Lodz University of Technology, Żeromskiego 116, 90-924 Łódź, Poland

Abstract

Polyenolate activation constitutes a powerful strategy, enabling the formation of higherenes. Alkylidenemalononitriles derived from indene-2-carbaldehydes upon deprotonation participate in a cascade involving [10 + 2]-cycloaddition followed by Michael addition and aldol condensation.

Funder

Narodowe Centrum Nauki

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/QO/D3QO02040A

Reference66 articles.

1. α,α-Dicyanoalkenes: versatile vinylogous nucleophiles for organic synthesis

2. Recent advances in organocatalytic asymmetric Michael reactions

3. The Vinylogous Aldol and Related Addition Reactions: Ten Years of Progress

4. New Developments of the Principle of Vinylogy as Applied to π-Extended Enolate-Type Donor Systems

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