Enhancing thermoelectric performance via relaxed spin polarization upon magnetic impurity doping

Author:

Kim Min Young1ORCID,Kim Dongwook2ORCID,Kim Gwansik3,Lee Wooyoung34ORCID,Perez Nicolas5,Nielsch Kornelius567,Shim Ji Hoon28,Jin Hyungyu19ORCID

Affiliation:

1. Department of Mechanical Engineering, Pohang University of Science and Technology (POSTECH), Pohang, 37673, South Korea

2. Department of Chemistry, Pohang University of Science and Technology (POSTECH), Pohang, 37673, South Korea

3. Department of Material Science and Engineering, Yonsei University, Seoul, 03722, South Korea

4. Affiliate Faculty, Materials Research Center for Batteries, Pohang University of Science and Technology (POSTECH), Pohang, 37673, South Korea

5. Leibniz Institute for Solid State and Materials Science, Dresden, 01069, Germany

6. Institute of Materials Science, TU Dresden, Dresden, 01062, Germany

7. Institute of Applied Physics, TU Dresden, Dresden, 01062, Germany

8. Division of Advanced Materials Science, Pohang University of Science and Technology (POSTECH), Pohang, 37673, South Korea

9. Institute for Convergence Research and Education in Advanced Technology, Yonsei University, Seoul, 03722, South Korea

Abstract

Here, a significant enhancement of the Seebeck coefficient is reported in magnetic-impurity-doped higher-manganese silicides, which is attributed to a magnetic-doping-induced relaxation of the spin-polarized band structure.

Funder

National Research Foundation of Korea

Ministry of Education

Ministry of Science and ICT, South Korea

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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