Boosting the synthesis of value-added aromatics directly from syngas via a Cr2O3 and Ga doped zeolite capsule catalyst

Author:

Wang Yang12345,Gao Weizhe678910,Wang Kangzhou678910,Gao Xinhua111213145ORCID,Zhang Baizhang678910,Zhao Heng678910,Ma Qingxiang111213145,Zhang Peipei678910,Yang Guohui678910ORCID,Wu Mingbo12345ORCID,Tsubaki Noritatsu678910ORCID

Affiliation:

1. College of New Energy

2. State Key Laboratory of Heavy Oil Processing

3. China University of Petroleum (East China)

4. Qingdao 266580

5. China

6. Department of Applied Chemistry

7. Graduate School of Engineering

8. University of Toyama

9. Toyama 930-8555

10. Japan

11. State Key Laboratory of High-efficiency Utilization of Coal and Green Chemical Engineering

12. College of Chemistry & Chemical Engineering

13. Ningxia University

14. Yinchuan 750021

Abstract

The single-pass conversion of syngas into para-xylene was realized using a bifunctional catalyst Cr2O3/Ga-ZSM-5@SiO2. The Ga species facilitates the methanol consumption process by C–C coupling optimization, enhancing the yield of the target aromatics.

Funder

Japan Science and Technology Agency

China Postdoctoral Science Foundation

China National Petroleum Corporation

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemistry

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