Screening of transition (Y, Zr, Hf, V, Nb, Mo, and Ru) and rare-earth (La and Pr) elements as potential effective dopants for thermoelectric GeTe – an experimental and theoretical appraisal

Author:

Srinivasan Bhuvanesh12345ORCID,Le Tonquesse Sylvain56783,Gellé Alain910111213,Bourgès Cédric1234,Monier Leo56783,Ohkubo Isao1234ORCID,Halet Jean-François56783ORCID,Berthebaud David56783ORCID,Mori Takao1234ORCID

Affiliation:

1. WPI International Center for Materials Nanoarchitectonics (WPI-MANA)

2. National Institute for Materials Science (NIMS)

3. Tsukuba 305-0044

4. Japan

5. CNRS-Saint Gobain-NIMS

6. UMI 3629

7. Laboratory for Innovative Key Materials and Structures (LINK)

8. National Institute for Materials Science

9. Univ. Rennes

10. CNRS

11. IPR

12. UMR 6251

13. F-35000 Rennes

Abstract

A report on an improvement in the thermoelectric performance of GeTe via intentional creation of more electrically dormant Ge vacancies (in contrast to classical approaches) and modulating/balancing it with optimized Zr-doping.

Funder

Japan Society for the Promotion of Science

Japan Science and Technology Agency

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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