Rational heterostructure stacking enables 23% wide-bandgap perovskite solar cells by side-reaction inhibition

Author:

Huang Tianyu1ORCID,Xu Fan12ORCID,Hu Jiangbing3,Wu Jiang3,Li Shunde1,Chen Peng1,Jia Xiaohan4,Li Qiuyang1,Yan Haoming1,Ji Yongqiang1,Luo Deying5ORCID,Wang Dengke6,Hu Juntao67,Chen Hao-Hsin1,Lu Zhangyuchang1,Xu Hongyu1,Li Lei1,Sha Rui3,Zhong Qixuan1,Bai Xinyu4ORCID,Dar M. Ibrahim4,Song Tinglu8ORCID,Li Zikun2,Yang Xiaoyu1,Zhao Lichen1ORCID,Lu Zheng-Hong56,Gong Qihuang139,Zhu Rui139ORCID

Affiliation:

1. State Key Laboratory for Artificial Microstructure and Mesoscopic Physics, School of Physics, Frontiers Science Center for Nano-optoelectronics & Collaborative Innovation Center of Quantum Matter, Peking University, Beijing, 100871, China

2. Shenzhen BTR New Energy Technology Institute Co., Ltd., Shenzhen, 518118, China

3. Peking University Yangtze Delta Institute of Optoelectronics, Nantong, 226010, China

4. Cavendish Laboratory, Department of Physics, University of Cambridge, Cambridge, CB3 0HE, UK

5. Department of Materials Science and Engineering, University of Toronto, Toronto, Ontario, M5S 2E8, Canada

6. Department of Physics, Center for Optoelectronics Engineering Research, Yunnan University, Kunming, 650091, China

7. Department of Physics, Mathematics and Computer Science, Faculty of Basic Medical Science, Kunming Medical University, Kunming, 650500, China

8. Experimental Centre for Advanced Materials, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, 100081, China

9. Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, 030006, China

Abstract

Suppressing side reactions led to the formation of rational Dion–Jacobson 2D/3D surface heterostructures, achieving an optimal PCE of 23.05% (certified 22.58%) for 1.68 eV perovskite solar cells.

Funder

Songshan Lake Materials Laboratory

Natural Science Foundation of Jiangsu Province

China Postdoctoral Science Foundation

National Natural Science Foundation of China

Beijing Nova Program

National Key Research and Development Program of China

Beijing Municipal Natural Science Foundation

Publisher

Royal Society of Chemistry (RSC)

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