Unravelling the carbonate issue through the regulation of mass transport and charge transfer in mild acid-Reference-Cited by-同舟云学术

Unravelling the carbonate issue through the regulation of mass transport and charge transfer in mild acid

Published:2024 Issue:8 Volume:15 Page:2786-2791
ISSN:2041-6520
Container-title:Chemical Science
language:en
Short-container-title:Chem. Sci.

Author:

Zhang Zhongshuo¹,Lu Qian¹²,Sun Jiping¹³,Li Guangchao¹³,Wu Weixing¹,Xu Zhanyou¹,Xu Liangpang¹,Wang Ying¹^ORCID

Affiliation:

1. Department of Chemistry, The Chinese University of Hong Kong, Hong Kong, S. A. R., China

2. Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, UNIST-NUIST Environment and Energy Jointed Lab, School of Environmental Science and Technology, Nanjing University of Information Science and Technology, Nanjing, P. R. China

3. School of Metallurgy and Environment, Central South University, Changsha, P. R. China

Abstract

Regulating the electrolyte hydrodynamics substantially reduces the proton diffusion length by 80%, which promotes the recovery of carbonate and leads to enhanced single-pass utilization of CO2 in mild acidic electrolyte.

Funder

National Natural Science Foundation of China

Research Grants Council, University Grants Committee

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/SC/D3SC06583A

Reference31 articles.

1. Electrochemical CO2-to-ethylene conversion on polyamine-incorporated Cu electrodes

2. Electrocatalytic reduction of CO2 to ethylene and ethanol through hydrogen-assisted C–C coupling over fluorine-modified copper

3. Suppression of Hydrogen Evolution in Acidic Electrolytes by Electrochemical CO2 Reduction

4. Competition between Hydrogen Evolution and Carbon Dioxide Reduction on Copper Electrodes in Mildly Acidic Media

5. CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface

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