An oxygen vacancy-rich two-dimensional Au/TiO2 hybrid for synergistically enhanced electrochemical N2 activation and reduction

Author:

Zhao Sen12345,Liu Han-Xuan67895,Qiu Yu12345,Liu Shuang-Quan12345,Diao Jin-Xiang12345,Chang Chun-Ran67895ORCID,Si Rui10115ORCID,Guo Xiao-Hui12345ORCID

Affiliation:

1. Key Lab of Synthetic and Natural Functional Molecule Chemistry of Ministry of Education

2. The College of Chemistry and Materials Science

3. Northwest University

4. Xi'an 710069

5. P. R. China

6. Shaanxi Key Laboratory of Energy Chemical Process Intensification

7. School of Chemical Engineering and Technology

8. Xi'an Jiaotong University

9. Xi'an 710049

10. Shanghai Synchrotron Radiation Facility Shanghai Institute of Applied Physics Chinese Academy of Sciences

11. Shanghai 201800

Abstract

An oxygen vacancy-rich Au/TiO2 hybrid nanosheet is used as an electrocatalyst for NRR that delivers a high NH3 yield of 64.6 μg h−1 mg−1 cat and an faradic efficiency (FE) of 29.5% and excellent structural stability under ambient conditions.

Funder

National Natural Science Foundation of China

China Postdoctoral Science Foundation

Fundamental Research Funds for the Central Universities

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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