Electrochemical conversion of bulk platinum into platinum single-atom sites for the hydrogen evolution reaction

Author:

Wang Zhiyuan12345,Yang Jia12345,Gan Jie6789,Chen Wenxing1011121314,Zhou Fangyao12345,Zhou Xiao12345,Yu Zhenqiang151617189ORCID,Zhu Junfa195209ORCID,Duan Xuezhi6789ORCID,Wu Yuen12345ORCID

Affiliation:

1. Hefei National Laboratory for Physical Sciences at the Microscale

2. Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)

3. School of Chemistry and Materials Science

4. National Synchrotron Radiation Laboratory

5. University of Science and Technology of China

6. State Key Laboratory of Chemical Engineering

7. East China University of Science and Technology

8. Shanghai 200237

9. China

10. Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications

11. School of Materials Science and Engineering

12. Beijing Institute of Technology

13. Beijing 100081

14. P. R. China

15. School of Chemistry and Environmental Engineering

16. Institute of Low-dimensional Materials Genome Initiative

17. Shenzhen University

18. Shenzhen 518060

19. National Synchrotron Radiation Laboratory (NSRL)

20. Hefei 230026

Abstract

An electro-filtration strategy is used to access a Pt single-atom sites catalyst on graphite carbon paper at room temperature from Pt foil, assisted by a GOM membrane. It exhibits excellent activity and stability towards HER (with CdS) under visible-light irradiation.

Funder

National Natural Science Foundation of China

China Postdoctoral Science Foundation

National Basic Research Program of China

Chinese Academy of Sciences

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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