Oxygen vacancy engineering in spinel-structured nanosheet wrapped hollow polyhedra for electrochemical nitrogen fixation under ambient conditions

Author:

Lai Feili12345,Feng Jianrui12345,Ye Xiaobin6789,Zong Wei12345,He Guanjie1011121314ORCID,Yang Chao151617189,Wang Wei151617189ORCID,Miao Yue-E.12345ORCID,Pan Bicai6789ORCID,Yan Wensheng6789,Liu Tianxi12345,Parkin Ivan P.1011121314ORCID

Affiliation:

1. State Key Laboratory for Modification of Chemical Fibers and Polymer Materials

2. College of Materials Science and Engineering

3. Innovation Center for Textile Science and Technology

4. Donghua University

5. Shanghai 201620

6. Hefei National Laboratory for Physical Sciences at the Microscale

7. University of Science and Technology of China

8. Hefei

9. P. R. China

10. Christopher Ingold Laboratory

11. Department of Chemistry

12. University College London

13. London WC1H 0AJ

14. UK

15. Department of Materials Science and Engineering

16. College of Engineering

17. Peking University

18. Beijing 100871

Abstract

Electrochemical nitrogen-to-ammonia conversion under ambient conditions is realized by an oxygen vacancy-rich spinel structured materials, showing relatively high faradaic efficiency and yields.

Funder

Engineering and Physical Sciences Research Council

National Natural Science Foundation of China

Science and Technology Commission of Shanghai Municipality

Program of Shanghai Academic Research Leader

Shanghai Education Development Foundation

Shanghai Municipal Education Commission

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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