Direct Z-scheme polymeric heterojunction boosts photocatalytic hydrogen production via a rebuilt extended π-delocalized network

Author:

Xu Linpeng1,Tian Bining1ORCID,Wang Tianyue12,Yu Ying2,Wu Yucheng13,Cui Jiewu3ORCID,Cao Zhongnan3,Wu Jianhong2,Zhang Weike1,Zhang Qi4ORCID,Liu Jiaqin4ORCID,Li Zhanfeng2ORCID,Tian Yue1ORCID

Affiliation:

1. Institute of New Carbon Materials, College of Materials Science and Engineering, Taiyuan University of Technology, Taiyuan 030024, China

2. Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education, College of Physics and Optoelectronics, Taiyuan University of Technology, Taiyuan 030024, China

3. Key Laboratory of Advanced Functional Materials and Devices of Anhui Province & School of Materials Science and Engineering, Hefei University of Technology, Hefei 230009, China

4. Institute of Industry & Equipment Technology, Hefei University of Technology, Hefei 230009, China

Abstract

We propose a strategy to rebuild the extended π-delocalized network in a Z-scheme polymeric heterojunction to improve the photon utilization efficiency, engendering an unprecedentedly high photocatalytic performance.

Funder

National Natural Science Foundation of China

Natural Science Foundation of Shanxi Province

Shanxi Scholarship Council of China

Fundamental Research Funds for the Central Universities

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Nuclear Energy and Engineering,Renewable Energy, Sustainability and the Environment,Environmental Chemistry

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