<i>Operando</i> investigations of the solid electrolyte interphase in the lithium mediated nitrogen reduction reaction-Reference-Cited by-同舟云学术

Operando investigations of the solid electrolyte interphase in the lithium mediated nitrogen reduction reaction

Published:2024 Issue:10 Volume:17 Page:3482-3492
ISSN:1754-5692
Container-title:Energy & Environmental Science
language:en
Short-container-title:Energy Environ. Sci.

Author:

Deissler Niklas H.¹^ORCID,Mygind J. Bjarke V.¹^ORCID,Li Katja¹^ORCID,Niemann Valerie A.²^ORCID,Benedek Peter²^ORCID,Vinci Valentin³,Li Shaofeng¹,Fu Xianbiao¹,Vesborg Peter C. K.¹^ORCID,Jaramillo Thomas F.²^ORCID,Kibsgaard Jakob¹^ORCID,Drnec Jakub³,Chorkendorff Ib¹^ORCID

Affiliation:

1. Department of Physics, Technical University of Denmark, Kongens Lyngby, Denmark

2. Department of Chemical Engineering, Stanford University, Stanford, CA, USA, SUNCAT Center for Interface Science and Catalysis, SLAC National Accelerator Laboratory, Menlo Park, CA, USA

3. Experimental Division, European Synchrotron Radiation Facility, Grenoble, France

Abstract

Operando GI-WAXS showed that the SEI layer formed by LiBF4 enhances Li-NRR performance by limiting proton transport to the electrode. Intermediate LiNxHy species give insight into the mechanism of Li-NRR.

Funder

Camille and Henry Dreyfus Foundation

HORIZON EUROPE Marie Sklodowska-Curie Actions

H2020 European Research Council

Innovationsfonden

Villum Fonden

National Science Foundation Graduate Research Fellowship Program

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/EE/D3EE04235A

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