An alternative approach towards poly-ε-caprolactone through a chemoenzymatic synthesis: combined hydrogenation, bio-oxidations and polymerization without the isolation of intermediates-Reference-Cited by-同舟云学术

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An alternative approach towards poly-ε-caprolactone through a chemoenzymatic synthesis: combined hydrogenation, bio-oxidations and polymerization without the isolation of intermediates

Published:2017 Issue:5 Volume:19 Page:1286-1290
ISSN:1463-9262
Container-title:Green Chemistry
language:en
Short-container-title:Green Chem.

Author:

Wedde Severin¹²³⁴⁵,Rommelmann Philipp¹²³⁴⁵,Scherkus Christian⁶⁷⁸⁵,Schmidt Sandy⁹¹⁰¹¹¹²⁵,Bornscheuer Uwe T.⁹¹⁰¹¹¹²⁵,Liese Andreas⁶⁷⁸⁵,Gröger Harald¹²³⁴⁵

Affiliation:

1. Chair of Organic Chemistry I

2. Faculty of Chemistry

3. Bielefeld University

4. 33615 Bielefeld

5. Germany

6. Institute of Technical Biocatalysis

7. Hamburg University of Technology

8. 21073 Hamburg

9. Institute of Biochemistry

10. Dept. of Biotechnology & Enzyme Catalysis

11. University of Greifswald

12. 17487 Greifswald

Abstract

A novel synthetic route towards the polymer poly-ε-caprolactone based on a chemoenzymatic reaction sequence was developed.

Funder

Deutsche Bundesstiftung Umwelt

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Environmental Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2017/GC/C6GC02529C

Reference34 articles.

1. Industrial Biotransformations, ed. A. Liese, K. Seelbach and C. Wandrey, Wiley-VCH, Weinheim, 2nd edn, 2006

2. Enzyme Catalysis in Organic Synthesis, ed. K. Drauz, H. Gröger and O. May, Wiley-VCH, Weinheim, 3rd edn, 2012, vol. 1–3

3. Process options for converting renewable feedstocks to bioproducts

4. Chemical Routes for the Transformation of Biomass into Chemicals

5. Chemicals from Renewables: Aerobic Oxidation of Furfural and Hydroxymethylfurfural over Gold Catalysts

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4. Development and Comparison of Substrate-Supplied and Product-Convergent Redox-Neutral Cascade Reactions for the Sustainable Synthesis of Lactones;ACS Sustainable Chemistry & Engineering;2023-07-05

5. Crosslinked Aggregates of Fusion Enzymes in Microaqueous Organic Media;ChemBioChem;2023-03-22

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