Enhancing electrocatalytic N2 reduction to NH3 by introducing Ni heteroatoms into NiCuOx electrocatalyst-Reference-Cited by-同舟云学术

Enhancing electrocatalytic N₂ reduction to NH₃ by introducing Ni heteroatoms into NiCuO_x electrocatalyst

Published:2024 Issue:13 Volume:14 Page:3691-3698
ISSN:2044-4753
Container-title:Catalysis Science & Technology
language:en
Short-container-title:Catal. Sci. Technol.

Author:

Han Xinxin¹^ORCID,Zhou Weizhen²,Huang Xin²,Yu Haoming²,Yang Fangqi³,Chen Shixia²^ORCID,Wang Jun²^ORCID

Affiliation:

1. School of Resources & Environment, Nanchang University, Nanchang 330031, People's Republic of China

2. School of Chemistry and Chemical Engineering, Nanchang University, Nanchang 330031, People's Republic of China

3. School of Materials Science and Engineering, Nanjing University of Posts and Telecommunications, Nanjing 210023, People's Republic of China

Abstract

The Ni dopant enhances the local electronic density surrounding Cu sites, which is favorable for reducing the energy barrier of the rate-determining (*N2 to *NNH) step of the NRR as well as depressing the competing HER.

Funder

Natural Science Foundation of Jiangxi Province

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/CY/D4CY00482E

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