Attosecond transient absorption spooktroscopy: a ghost imaging approach to ultrafast absorption spectroscopy

Author:

Driver Taran12323ORCID,Li Siqi23453ORCID,Champenois Elio G.123,Duris Joseph23,Ratner Daniel23,Lane Thomas J.23,Rosenberger Philipp12367,Al-Haddad Andre89,Averbukh Vitali1041112,Barnard Toby1041112,Berrah Nora13143ORCID,Bostedt Christoph89159,Bucksbaum Philip H.12345,Coffee Ryan12323,DiMauro Louis F.4163,Fang Li4163,Garratt Douglas1041112,Gatton Averell23,Guo Zhaoheng12345,Hartmann Gregor17187197,Haxton Daniel203,Helml Wolfram21227ORCID,Huang Zhirong23453,LaForge Aaron13143ORCID,Kamalov Andrei12345,Kling Matthias F.12367ORCID,Knurr Jonas123,Lin Ming-Fu23,Lutman Alberto A.23,MacArthur James P.23453,Marangos Jon P.1041112,Nantel Megan23453,Natan Adi123,Obaid Razib13143ORCID,O'Neal Jordan T.12345,Shivaram Niranjan H.23ORCID,Schori Aviad123,Walter Peter23,Li Wang Anna123235,Wolf Thomas J. A.123ORCID,Marinelli Agostino23,Cryan James P.12323ORCID

Affiliation:

1. Stanford PULSE Institute

2. SLAC National Accelerator Laboratory

3. USA

4. Department of Physics

5. Stanford University

6. Max-Planck-Institut für Quantenoptik

7. Germany

8. Paul Scherrer Institut

9. Switzerland

10. The Blackett Laboratory

11. Imperial College London

12. UK

13. Physics Department

14. University of Connecticut

15. LUXS Laboratory for Ultrafast X-ray Sciences, École Polytechnique Fédérale de Lausanne

16. The Ohio State University

17. Institut für Physik und CINSaT

18. Universität Kassel

19. Helmholtz-Zentrum Berlin

20. KLA Tencor Corporation

21. Zentrum für Synchrotronstrahlung

22. Technische Universität Dortmund

23. Department of Applied Physics

Abstract

Recently demonstrated isolated attosecond XFEL pulses should allow the probing of ultrafast electron dynamics at X-ray wavelengths. The authors use ghost imaging to enable high-resolution transient absorption spectroscopy at fluctuating XFEL sources.

Funder

Basic Energy Sciences

Deutsche Forschungsgemeinschaft

Engineering and Physical Sciences Research Council

National Science Foundation

SLAC National Accelerator Laboratory

Max-Planck-Gesellschaft

Chemical Sciences, Geosciences, and Biosciences Division

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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