1. Department of Civil and Environmental Engineering, University of California, Irvine, Irvine, California 92697-2175, Department of Chemistry and Biochemistry, and Center for Marine Science, University of North Carolina Wilmington, 5600 Marvin K. Moss Lane, Wilmington, North Carolina 28409, and Marine and Atmospheric Chemistry, Rosenstiel School of Marine and Atmospheric Sciences, University of Miami, 4600 Rickenbacker Causeway, Miami, Florida 33149